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Electron Spin Manipulation via Encaged Cluster: Differing Anion Radicals of Y-2@C-82-C-s, Y2C2@C-82-C-s, and Sc2C2@C-82-C-s
Ma, YH; Wang, TS; 吴静怡; Wu, JY; Feng, YQ; Li, H; Jiang, L; Shu, CY; Wang, CR
2013
发表期刊JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷号4期号:3页码:464-467
摘要Endohedral metallofullerene species with controllable electron spin have attracted increasing attention along with their potential application in quantum information processing. In this paper, we report the electron spin manipulation via encage cluster through comparative studies on the anion radicals of metallofullerene Y-2@C-82-C-s, Y2C2@C-82-C-s, and Sc2C2@C-82-C-s. Although these three radical species have the same parent fullerene cage, we found that the unpaired spin characteristics as well as metal-spin couplings of them can be greatly affected by endohedral clusters. Furthermore, based on theoretical calculations, it was revealed that the encaged clusters can affect the electronic population of pristine endohedral metallofullerenes and eventually manipulate the spin distribution of their corresponding anion radicals. Our findings are referential to the spin coherence in information processing due to the variable paramagnetism of these metallofullerene radicals.
学科领域Chemistry; Science & Technology - Other Topics; Materials Science; Physics
DOI10.1021/jz3020666
收录类别SCI
WOS记录号WOS:000314907500022
引用统计
被引频次:11[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/223990
专题多学科研究中心
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GB/T 7714
Ma, YH,Wang, TS,吴静怡; Wu, JY,et al. Electron Spin Manipulation via Encaged Cluster: Differing Anion Radicals of Y-2@C-82-C-s, Y2C2@C-82-C-s, and Sc2C2@C-82-C-s[J]. JOURNAL OF PHYSICAL CHEMISTRY LETTERS,2013,4(3):464-467.
APA Ma, YH.,Wang, TS.,吴静怡; Wu, JY.,Feng, YQ.,Li, H.,...&Wang, CR.(2013).Electron Spin Manipulation via Encaged Cluster: Differing Anion Radicals of Y-2@C-82-C-s, Y2C2@C-82-C-s, and Sc2C2@C-82-C-s.JOURNAL OF PHYSICAL CHEMISTRY LETTERS,4(3),464-467.
MLA Ma, YH,et al."Electron Spin Manipulation via Encaged Cluster: Differing Anion Radicals of Y-2@C-82-C-s, Y2C2@C-82-C-s, and Sc2C2@C-82-C-s".JOURNAL OF PHYSICAL CHEMISTRY LETTERS 4.3(2013):464-467.
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