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Fe-N4 Doped Carbon Nanotube Cathode Catalyst for PEM Fuel Cells | |
BSRF用户 | |
2021 | |
Source Publication | ACS APPLIED MATERIALS & INTERFACES
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ISSN | 1944-8244 |
EISSN | 1944-8252 |
Volume | 13Issue:41Pages:48923--48933 |
Subtype | Article |
Abstract | The earth-abundant iron and nitrogen doped carbon (Fe-N-C) catalyst has great potential to substitute noble metal catalysts for oxygen reduction reaction (ORR) in H-2-O-2 proton exchange membrane fuel cells (PEMFCs). Herein, we report the preparation of Fe-N-4 moiety doped carbon nanotubes (CNTs) by ball milling and two-step pyrolysis with dual metal-organic frameworks (MOFs) as the precursor. This catalyst shows high ORR catalytic performance and stability. Different from traditional inorganic iron sources, the MOF structure can effectively prevent the iron metal from aggregating during pyrolysis. In PEMFC, the catalyst shows high current density (0.39 A/cm(2) at 0.7 V) and power density (850 mW/cm(2)). Such a method brings inspiration for the reasonable design of FeNC catalysts with high catalytic activity for H-2-O-2 PEMFCs. |
DOI | 10.1021/acsami.1c15554 |
Indexed By | SCI |
Language | 英语 |
WOS Research Area | Science & Technology - Other Topics ; Materials Science |
WOS Subject | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
WOS ID | WOS:000710924900057 |
ItemNo | BSRF00747 |
beamline | 4B9A |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.ihep.ac.cn/handle/311005/293515 |
Collection | 北京同步辐射装置 |
Recommended Citation GB/T 7714 | BSRF用户. Fe-N4 Doped Carbon Nanotube Cathode Catalyst for PEM Fuel Cells[J]. ACS APPLIED MATERIALS & INTERFACES,2021,13(41):48923--48933. |
APA | BSRF用户.(2021).Fe-N4 Doped Carbon Nanotube Cathode Catalyst for PEM Fuel Cells.ACS APPLIED MATERIALS & INTERFACES,13(41),48923--48933. |
MLA | BSRF用户."Fe-N4 Doped Carbon Nanotube Cathode Catalyst for PEM Fuel Cells".ACS APPLIED MATERIALS & INTERFACES 13.41(2021):48923--48933. |
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