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Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition
Cheng, XY; Zhang, BX; Shi, JB; Zhang, JL; Zheng, LR; Zhang, J; Shao, D; Tan, XN; Han, BX; Yang, GY; Zheng LR(郑黎荣); Zhang J(张静)
2018
Source PublicationCHEMCATCHEM
ISSN1867-3880
EISSN1867-3899
Volume10Issue:14Pages:2945-2948
SubtypeArticle
AbstractTo overcome the limitations of metal-organic frameworks (MOFs) for catalysis (e.g., low catalytic activities resulting from blockage of the active metal centers by organic linkers) is of great importance. Herein, we demonstrate the formation of UiO-66 nanoparticles with ultrasmall size and linker defects with the aid of SnS2 nanosheets. The UiO-66 nanoparticles supported by SnS2 nanosheets were found to exhibit excellent catalytic activity for the cycloaddition reaction of CO2 with propylene oxide under solvent-free and co-catalyst-free conditions. Outstandingly, the catalytic activity was 11times higher than that of the pure UiO-66 catalyst under optimum conditions. We thus provide a promising route to modify MOF particles thus to promote their catalytic performance.
Keywordcycloaddition heterogeneous catalysis metal-organic frameworks nanoparticles tin sulfide
DOI10.1002/cctc.201800411
WOS KeywordMETAL-ORGANIC FRAMEWORKS ; CYCLIC CARBONATES ; HETEROGENEOUS CATALYSTS ; CO2 ; EPOXIDES ; TRANSFORMATION ; NANOSHEETS ; DESIGN
Indexed BySCI ; EI
Language英语
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
WOS IDWOS:000439756600003
EI Accession Number20183005589696
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ihep.ac.cn/handle/311005/286256
Collection多学科研究中心
实验物理中心
Affiliation中国科学院高能物理研究所
First Author AffilicationInstitute of High Energy
Recommended Citation
GB/T 7714
Cheng, XY,Zhang, BX,Shi, JB,et al. Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition[J]. CHEMCATCHEM,2018,10(14):2945-2948.
APA Cheng, XY.,Zhang, BX.,Shi, JB.,Zhang, JL.,Zheng, LR.,...&张静.(2018).Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition.CHEMCATCHEM,10(14),2945-2948.
MLA Cheng, XY,et al."Tin(IV) Sulfide Greatly Improves the Catalytic Performance of UiO-66 for Carbon Dioxide Cycloaddition".CHEMCATCHEM 10.14(2018):2945-2948.
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