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Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance
Liu, W; Xu, Q; Yan, PF; Chen, J; Du, Y; Chu, SQ; Wang, JO; Chu SQ(储胜启); Wang JO(王嘉鸥)
2018
Source PublicationCHEMCATCHEM
ISSN1867-3880
EISSN1867-3899
Volume10Issue:5Pages:946-950
SubtypeArticle
AbstractSingle-atom catalysts (SACs) play a key role in many chemical processes owing to highly desirable atom efficiency, but the challenging synthesis of these catalysts limits their commercialization and application on a large scale. Herein, we report a facile strategy to integrate atomic Pt into richly deficient MoO3-x. The core of the experimental strategy was the fabrication and utilization of HxMoO3-x with plasmon resonance that contained intercalated H+. The obtained catalyst was found to possess remarkable electrocatalytic activity toward the hydrogen evolution reaction that was even comparable to that of commercial Pt/C, whereas the amount of Pt used was reduced to only 10% of the amount of commercial Pt/C used. Therefore, this work not only supplies a new synthesis route to SACs but also reveals the potential relation between plasmon resonance materials and the fabrication of single-atom catalysts.
Keywordamorphous materials hydrogen molybdenum surface plasmon resonance single-atom catalysts
DOI10.1002/cctc.201701777
WOS KeywordCO OXIDATION ; EFFICIENT ; NANOSHEETS ; PERFORMANCE ; ALPHA-MOO3 ; GRAPHENE ; CLUSTERS ; SURFACE ; H-MOO3 ; WATER
Indexed BySCI ; EI
Language英语
WOS Research AreaChemistry
WOS SubjectChemistry, Physical
WOS IDWOS:000426844600009
EI Accession Number20180604770041
Citation statistics
Document Type期刊论文
Identifierhttp://ir.ihep.ac.cn/handle/311005/285712
Collection粒子天体物理中心
多学科研究中心
Affiliation中国科学院高能物理研究所
First Author AffilicationInstitute of High Energy
Recommended Citation
GB/T 7714
Liu, W,Xu, Q,Yan, PF,et al. Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance[J]. CHEMCATCHEM,2018,10(5):946-950.
APA Liu, W.,Xu, Q.,Yan, PF.,Chen, J.,Du, Y.,...&王嘉鸥.(2018).Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance.CHEMCATCHEM,10(5),946-950.
MLA Liu, W,et al."Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance".CHEMCATCHEM 10.5(2018):946-950.
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