| Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance | |
Liu, W; Xu, Q ; Yan, PF; Chen, J; Du, Y; Chu, SQ; Wang, JO; Chu SQ(储胜启); Wang JO(王嘉鸥)
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| 2018 | |
| Source Publication | CHEMCATCHEM
 |
| ISSN | 1867-3880 |
| EISSN | 1867-3899 |
| Volume | 10Issue:5Pages:946-950 |
| Subtype | Article |
| Abstract | Single-atom catalysts (SACs) play a key role in many chemical processes owing to highly desirable atom efficiency, but the challenging synthesis of these catalysts limits their commercialization and application on a large scale. Herein, we report a facile strategy to integrate atomic Pt into richly deficient MoO3-x. The core of the experimental strategy was the fabrication and utilization of HxMoO3-x with plasmon resonance that contained intercalated H+. The obtained catalyst was found to possess remarkable electrocatalytic activity toward the hydrogen evolution reaction that was even comparable to that of commercial Pt/C, whereas the amount of Pt used was reduced to only 10% of the amount of commercial Pt/C used. Therefore, this work not only supplies a new synthesis route to SACs but also reveals the potential relation between plasmon resonance materials and the fabrication of single-atom catalysts. |
| Keyword | amorphous materials hydrogen molybdenum surface plasmon resonance single-atom catalysts |
| DOI | 10.1002/cctc.201701777 |
| WOS Keyword | CO OXIDATION ; EFFICIENT ; NANOSHEETS ; PERFORMANCE ; ALPHA-MOO3 ; GRAPHENE ; CLUSTERS ; SURFACE ; H-MOO3 ; WATER |
| Indexed By | SCI ; EI |
| Language | 英语 |
| WOS Research Area | Chemistry |
| WOS Subject | Chemistry, Physical |
| WOS ID | WOS:000426844600009 |
| EI Accession Number | 20180604770041 |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.ihep.ac.cn/handle/311005/285712 |
| Collection | 粒子天体物理中心 多学科研究中心 |
| Affiliation | 中国科学院高能物理研究所 |
| First Author Affilication | Institute of High Energy |
| Recommended Citation GB/T 7714 | Liu, W,Xu, Q,Yan, PF,et al. Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance[J]. CHEMCATCHEM,2018,10(5):946-950. |
| APA | Liu, W.,Xu, Q.,Yan, PF.,Chen, J.,Du, Y.,...&王嘉鸥.(2018).Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance.CHEMCATCHEM,10(5),946-950. |
| MLA | Liu, W,et al."Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of HxMoO3-x with Plasmon Resonance".CHEMCATCHEM 10.5(2018):946-950. |
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