Formation of Ordered Coronene Clusters in Template Utilizing the Structural Transformation of Hexaphenylbenzene Derivative Networks on Graphite Surface
Chang, SQ; Liu RC(刘润聪); Liu, RC; Wang, LC; Li M(李敏); Li, M; Deng, K; Zheng, QY; Zeng, QD
刊名ACS NANO
2016
卷号10期号:1页码:342-348
关键词structural transformation HPB network coronene cluster scanning tunneling microscopy guest inclusion
DOI10.1021/acsnano.5b06666
通讯作者李敏
文章类型期刊论文
英文摘要In the present work, we report the fabrication of regular coronene (COR) clusters on surfaces in ambient conditions in the two-dimensional network formed by hexaphenylbenzene derivatives (HPB) via structural transformation. HPB could form a stable snowflake network structure on the highly oriented pyrolytic graphite surface at the air solid interface. When COR molecules were introduced into the system, the HPB snowflake network could transform to honeycomb structures, and the COR heptamers were subsequently aggregated and entrapped into the cavity. Scanning tunneling microscopic was employed to monitor the assembly behavior of both HPB and HPB/COR at a submolecule scale level, and density functional theory calculations were utilized to reveal that the structural transformation and the entrapment are the energetically favorable. The pores formed from HPB might also give a clue to immobilizing some functional molecule clusters, like COR, to fabricate their ordered monolayer in ambient conditions, so as to obtain complex supramolecular surface structures.
类目[WOS]Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
关键词[WOS]LIQUID-SOLID INTERFACE ; GUEST INCLUSION ; MANIPULATION ; ORGANIZATION ; ASSEMBLIES ; ADSORPTION ; MOLECULES ; AU(111) ; SYSTEMS
语种英语
WOS记录号WOS:000369115800035
引用统计
被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/260375
专题中国科学院高能物理研究所_多学科研究中心_期刊论文
中国科学院高能物理研究所_多学科研究中心
作者单位中国科学院高能物理研究所
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GB/T 7714
Chang, SQ,Liu RC,Liu, RC,et al. Formation of Ordered Coronene Clusters in Template Utilizing the Structural Transformation of Hexaphenylbenzene Derivative Networks on Graphite Surface[J]. ACS NANO,2016,10(1):342-348.
APA Chang, SQ.,刘润聪.,Liu, RC.,Wang, LC.,李敏.,...&Zeng, QD.(2016).Formation of Ordered Coronene Clusters in Template Utilizing the Structural Transformation of Hexaphenylbenzene Derivative Networks on Graphite Surface.ACS NANO,10(1),342-348.
MLA Chang, SQ,et al."Formation of Ordered Coronene Clusters in Template Utilizing the Structural Transformation of Hexaphenylbenzene Derivative Networks on Graphite Surface".ACS NANO 10.1(2016):342-348.
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