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Metal-Organic Framework for Emulsifying Carbon Dioxide and Water
Liu, CC; Zhang, JL; Zheng, L; Zhang, J; Sang, XX; Kang, XC; Zhang, BX; Luo, T; Tan, XN; Han, BX; Zheng LR(郑黎荣); Zhang J(张静)
2016
发表期刊ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷号55期号:38页码:11372-11376
文章类型期刊论文
摘要Forming emulsions of carbon dioxide (CO2) and water can largely expand the utility of CO2. Herein we propose for the first time the utilization of a metal-organic framework (MOF) for emulsifying CO2 and water. Owing to the hybrid composition, MOF particles can easily assemble at the CO2/water interface to create a rigid protective barrier around the dispersed droplet. The MOF-stabilized CO2 and water emulsion has exceptional stability compared to those emulsions stabilized by surfactants or other solids. Moreover, the CO2 and water emulsion stabilized by MOF is tunable due to the designable features of MOFs and adjustable character of CO2. Such a novel kind of emulsion composed of CO2, water, and MOF provides a facile route for constructing MOF superstructures with many advantages. The macroporous networks and hollow capsules of different kinds of MOFs have been successfully derived from CO2 and water emulsions.
关键词CO2 emulsions H2O metal-organic frameworks superstructures
DOI10.1002/anie.201602150
关键词[WOS]PICKERING EMULSIONS ; STUBBY SURFACTANTS ; COMPRESSED CO2 ; STABILIZATION ; ADSORPTION ; GAS ; PARTICLES ; INTERFACE ; COLLOIDS ; POLYMER
语种英语
WOS类目Chemistry, Multidisciplinary
WOS记录号WOS:000383748900006
引用统计
被引频次:10[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/260330
专题多学科研究中心
作者单位中国科学院高能物理研究所
推荐引用方式
GB/T 7714
Liu, CC,Zhang, JL,Zheng, L,et al. Metal-Organic Framework for Emulsifying Carbon Dioxide and Water[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2016,55(38):11372-11376.
APA Liu, CC.,Zhang, JL.,Zheng, L.,Zhang, J.,Sang, XX.,...&张静.(2016).Metal-Organic Framework for Emulsifying Carbon Dioxide and Water.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,55(38),11372-11376.
MLA Liu, CC,et al."Metal-Organic Framework for Emulsifying Carbon Dioxide and Water".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 55.38(2016):11372-11376.
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