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Determination of the sites of Fe atoms in Fe-substituted Mn-12
Cao, HB; Chen DL(陈栋梁); Wu ZY(吴自玉); Chen, DL; He, LH; Zhang, JR; Wang, FW; Wu, ZY; Yan, QW
2007
发表期刊CHINESE PHYSICS
卷号16期号:3页码:784-787
通讯作者Chinese Acad Sci, Inst Phys, State Key Lab Magnetism, Beijing 100080, Peoples R China ; Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China
文章类型Article
摘要In this paper neutron diffraction experiments were performed for Fe-substituted Mn-12 in order to determine the sites of Fe atoms. The results of structure refinements for the sample with our accessed highest Fe content showed that all Fe atoms occupied Mn(3) sites in the Mn-12 skeleton. The x-ray absorption. ne structure experiments as well as multiple scattering simulations gave the same result. Thus we concluded that Fe atoms only occupied Mn( 3) sites. This conclusion also means that Fe-substituted Mn-12 series only includes the four single-molecule magnets of [Mn(12-x)FexO(12)(CH3COO)(16)(H2O)(4)] center dot 2CH(3)COOH center dot 4H(2)O (x = 1, 2, 3, and 4), denoted by Mn11Fe1, Mn10Fe2, Mn9Fe3, and Mn8Fe4, respectively.
关键词single-molecule magnets neutron diffraction x-ray absorption fine structure
学科领域Physics
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语种英语
WOS研究方向Physics
WOS类目Physics, Multidisciplinary
WOS记录号WOS:000244864500037
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被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/238481
专题多学科研究中心
作者单位中国科学院高能物理研究所
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Cao, HB,Chen DL,Wu ZY,et al. Determination of the sites of Fe atoms in Fe-substituted Mn-12[J]. CHINESE PHYSICS,2007,16(3):784-787.
APA Cao, HB.,陈栋梁.,吴自玉.,Chen, DL.,He, LH.,...&Yan, QW.(2007).Determination of the sites of Fe atoms in Fe-substituted Mn-12.CHINESE PHYSICS,16(3),784-787.
MLA Cao, HB,et al."Determination of the sites of Fe atoms in Fe-substituted Mn-12".CHINESE PHYSICS 16.3(2007):784-787.
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