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The NuSTAR View of a QPO Evolution of GRS 1915+105
Zhang; L.; L. Chen; Qu JL(屈进禄); J.-l. Qu; Q.-C. Bu
2015
发表期刊The Astronomical Journal
卷号54期号:22页码:10934-10945
摘要A unique case of a uranyl-silver heterometallic 3-fold interpenetrating network (U-Ag-2,6-DCPCA) from a multifunctionalized organic ligand, 2,6-dichloroisonicotinic acid, in the presence of uranyl and silver ions is reported. It is the first report of a heterometallic uranylorganic interpenetrating network or framework. Notably, a (4,4)-connected uranyl building unit in U-Ag-2,6-DCPCA, which is available through combined influences of structural halogenation and silver ion additive on uranyl coordination, plays a vital role in the formation of a 3-fold interpenetrating network. Halogen substitution effectively changes structural features and coordination behaviors of isonicotinate ligand and contributes to the control of uranyl coordination. Meanwhile, it exerts influence on the stabilization of 3-fold interpenetrating networks by halogen-halogen interactions. Theoretical calculation suggests that the silver ion should mainly serve as an inductive factor of uranyl species through strong Ag-N binding affinity, directly leading to the formation of a (4,4)-connected uranyl building unit and finally a heterometallic 3-fold interpenetrating network. Related experimental results, especially an interesting postsynthetic metalation, afford further evidence of this induction effect.
文章类型Article
学科领域Chemistry
DOI10.1021/acs.inorgchem.5b01988
收录类别SCI
WOS类目Chemistry, Inorganic & Nuclear
WOS记录号WOS:000364981300052
引用统计
被引频次:19[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/228956
专题粒子天体物理中心
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Zhang,L.,L. Chen,et al. The NuSTAR View of a QPO Evolution of GRS 1915+105[J]. The Astronomical Journal,2015,54(22):10934-10945.
APA Zhang,L.,L. Chen,屈进禄,J.-l. Qu,&Q.-C. Bu.(2015).The NuSTAR View of a QPO Evolution of GRS 1915+105.The Astronomical Journal,54(22),10934-10945.
MLA Zhang,et al."The NuSTAR View of a QPO Evolution of GRS 1915+105".The Astronomical Journal 54.22(2015):10934-10945.
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