IHEP OpenIR
Local atomic structure modulations activate metal oxide as electrocatalyst for hydrogen evolution in acidic water
Li, YH; Liu, PF; Pan, LF; Wang, HF; Yang, ZZ; Zheng, LR; Hu, P; Zhao, HJ; Gu, L; Yang, HG; Zheng LR(郑黎荣)
2015
Source PublicationNATURE COMMUNICATIONS
ISSN2041-1723
Volume6Pages:8064
SubtypeArticle
AbstractModifications of local structure at atomic level could precisely and effectively tune the capacity of materials, enabling enhancement in the catalytic activity. Here we modulate the local atomic structure of a classical but inert transition metal oxide, tungsten trioxide, to be an efficient electrocatalyst for hydrogen evolution in acidic water, which has shown promise as an alternative to platinum. Structural analyses and theoretical calculations together indicate that the origin of the enhanced activity could be attributed to the tailored electronic structure by means of the local atomic structure modulations. We anticipate that suitable structure modulations might be applied on other transition metal oxides to meet the optimal thermodynamic and kinetic requirements, which may pave the way to unlock the potential of other promising candidates as cost-effective electrocatalysts for hydrogen evolution in industry.
Subject AreaScience & Technology - Other Topics
DOI10.1038/ncomms9064
Indexed BySCI ; ADS
Language英语
WOS Research AreaMultidisciplinary Sciences
WOS SubjectScience & Technology - Other Topics
WOS IDWOS:000360353000001
ADS Bibcode2015NatCo...6.8064L
ADS URLhttps://ui.adsabs.harvard.edu/abs/2015NatCo...6.8064L
ADS CITATIONShttps://ui.adsabs.harvard.edu/abs/2015NatCo...6.8064L/citations
Citation statistics
Cited Times:46 [ADS]
Document Type期刊论文
Identifierhttp://ir.ihep.ac.cn/handle/311005/228758
Collection中国科学院高能物理研究所
Recommended Citation
GB/T 7714
Li, YH,Liu, PF,Pan, LF,et al. Local atomic structure modulations activate metal oxide as electrocatalyst for hydrogen evolution in acidic water[J]. NATURE COMMUNICATIONS,2015,6:8064.
APA Li, YH.,Liu, PF.,Pan, LF.,Wang, HF.,Yang, ZZ.,...&郑黎荣.(2015).Local atomic structure modulations activate metal oxide as electrocatalyst for hydrogen evolution in acidic water.NATURE COMMUNICATIONS,6,8064.
MLA Li, YH,et al."Local atomic structure modulations activate metal oxide as electrocatalyst for hydrogen evolution in acidic water".NATURE COMMUNICATIONS 6(2015):8064.
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