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Local atomic structure modulations activate metal oxide as electrocatalyst for hydrogen evolution in acidic water
Li, YH; Liu, PF; Pan, LF; Wang, HF; Yang, ZZ; Zheng, LR; Hu, P; Zhao, HJ; Gu, L; Yang, HG; Zheng LR(郑黎荣)
2015
发表期刊NATURE COMMUNICATIONS
卷号6页码:8064
文章类型Article
摘要Modifications of local structure at atomic level could precisely and effectively tune the capacity of materials, enabling enhancement in the catalytic activity. Here we modulate the local atomic structure of a classical but inert transition metal oxide, tungsten trioxide, to be an efficient electrocatalyst for hydrogen evolution in acidic water, which has shown promise as an alternative to platinum. Structural analyses and theoretical calculations together indicate that the origin of the enhanced activity could be attributed to the tailored electronic structure by means of the local atomic structure modulations. We anticipate that suitable structure modulations might be applied on other transition metal oxides to meet the optimal thermodynamic and kinetic requirements, which may pave the way to unlock the potential of other promising candidates as cost-effective electrocatalysts for hydrogen evolution in industry.
学科领域Science & Technology - Other Topics
DOI10.1038/ncomms9064
收录类别SCI
WOS类目Multidisciplinary Sciences
WOS记录号WOS:000360353000001
引用统计
被引频次:74[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/228758
专题多学科研究中心
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GB/T 7714
Li, YH,Liu, PF,Pan, LF,et al. Local atomic structure modulations activate metal oxide as electrocatalyst for hydrogen evolution in acidic water[J]. NATURE COMMUNICATIONS,2015,6:8064.
APA Li, YH.,Liu, PF.,Pan, LF.,Wang, HF.,Yang, ZZ.,...&郑黎荣.(2015).Local atomic structure modulations activate metal oxide as electrocatalyst for hydrogen evolution in acidic water.NATURE COMMUNICATIONS,6,8064.
MLA Li, YH,et al."Local atomic structure modulations activate metal oxide as electrocatalyst for hydrogen evolution in acidic water".NATURE COMMUNICATIONS 6(2015):8064.
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