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The decolorization of Acid Orange II in non-homogeneous Fenton reaction catalyzed by natural vanadium-titanium magnetite
Liang, XL; Zhong, YH; Zhu, SY; Zhu, JX; Yuan, P; He, HP; Zhang, J; Zhang J(张静)
2010
发表期刊JOURNAL OF HAZARDOUS MATERIALS
卷号181期号:1-3页码:#REF!
通讯作者He, HP (reprint author), Chinese Acad Sci, Guangzhou Inst Geochem, Guangzhou 510640, Peoples R China.
文章类型Article
摘要The catalytic activity of natural vanadium-titanium magnetite was investigated in the decolorization of Acid Orange II by non-homogeneous Fenton process. The natural catalysts purified by magnetic separation were characterized using X-ray diffraction (XRD), polarizing microscope. X-ray absorption fine structure (XAFS) analysis and Mossbauer spectroscopy. The obtained results show that the natural samples after magnetic separation mainly contain titanomagnetite, with a small amount of ilmenite and chlorite. Titanomagnetite is doped with vanadium, whose the valency is mainly +3 and occupies the octahedral site. Batch decolorization studies were performed to evaluate the influences of various experimental parameters like initial pH, the amount of catalyst and initial concentration of hydrogen peroxide on the decolorization efficiency of Acid Orange II. The decolorization of the dye mainly relied on degradation. The degradation efficiency was strongly dependent on pH of the medium where it increased as the pH decreased in acid range. The increase of catalyst and hydrogen peroxide could accelerate the degradation. The catalytic property of natural vanadium-titanium magnetite in the degradation of Acid Orange II was stronger than that of synthetic magnetite (Fe(3)O(4)). The catalytic activity of the natural samples was greatly related to the titanomagnetite content. The degradation process was dominated by heterogeneous Fenton reaction, complying with pseudo-first-order rate law. The natural catalyst has a good catalytic stability. (C) 2010 Elsevier B.V. All rights reserved.
关键词Natural vanadium-titanium magnetite Non-homogeneous Fenton reaction Degradation Acid Orange II Catalyst
学科领域Engineering; Environmental Sciences & Ecology
DOI10.1016/j.jhazmat.2010.04.101
收录类别SCI
WOS类目Engineering, Environmental ; Engineering, Civil ; Environmental Sciences
WOS记录号WOS:000280601300014
引用统计
被引频次:73[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/226239
专题多学科研究中心
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GB/T 7714
Liang, XL,Zhong, YH,Zhu, SY,et al. The decolorization of Acid Orange II in non-homogeneous Fenton reaction catalyzed by natural vanadium-titanium magnetite[J]. JOURNAL OF HAZARDOUS MATERIALS,2010,181(1-3):#REF!.
APA Liang, XL.,Zhong, YH.,Zhu, SY.,Zhu, JX.,Yuan, P.,...&张静.(2010).The decolorization of Acid Orange II in non-homogeneous Fenton reaction catalyzed by natural vanadium-titanium magnetite.JOURNAL OF HAZARDOUS MATERIALS,181(1-3),#REF!.
MLA Liang, XL,et al."The decolorization of Acid Orange II in non-homogeneous Fenton reaction catalyzed by natural vanadium-titanium magnetite".JOURNAL OF HAZARDOUS MATERIALS 181.1-3(2010):#REF!.
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