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Highly efficient photodimerization of olefins in a nanotemplate on HOPG by scanning tunneling microscopy
Xue, JD; Xu, J; Hu, FY; Liao, LY; Li, M; Duan, WB; Zeng, QD; Wang, C;李敏
2014
发表期刊PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷号16期号:47页码:25765-25769
摘要Efficient photochemical reactions on a surface are of great importance for their potential applications in optoelectronic devices. In this work, a highly efficient photodimerization reaction of an olefin cocrystal built from two trans-1,2-bis(4-pyridyl) ethylenes (4,4'-bpe) and two isophthalic acid molecules via N center dot center dot center dot H-O hydrogen bonds in between was achieved in a nanotemplate on a highly oriented pyrolytic graphite (HOPG) surface. 4,4'-Bpe molecules first undergo the trans-cis isomerization followed by [2+2] photodimerization in the nanotemplate on HOPG upon UV irradiation. The efficiency of the isomerization as well as the photodimerization in the presence of the nanotemplate is much higher than that in its absence. These results provide a facile way to achieve highly efficient photodimerization of olefins on a large scale on surfaces.
学科领域Chemistry; Physics
DOI10.1039/c4cp04154b
收录类别SCI
WOS记录号WOS:000345208200013
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被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/225254
专题多学科研究中心
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Xue, JD,Xu, J,Hu, FY,et al. Highly efficient photodimerization of olefins in a nanotemplate on HOPG by scanning tunneling microscopy[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2014,16(47):25765-25769.
APA Xue, JD.,Xu, J.,Hu, FY.,Liao, LY.,Li, M.,...&Wang, C;李敏.(2014).Highly efficient photodimerization of olefins in a nanotemplate on HOPG by scanning tunneling microscopy.PHYSICAL CHEMISTRY CHEMICAL PHYSICS,16(47),25765-25769.
MLA Xue, JD,et al."Highly efficient photodimerization of olefins in a nanotemplate on HOPG by scanning tunneling microscopy".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 16.47(2014):25765-25769.
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