One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel
Kang, XC; Zhang, JL; Shang, WT; Wu, TB; Zhang, P; Han, BX; Wu, ZH; Mo, G; Xing, XQ;吴忠华; Mo G(默广); Xing XQ(邢雪青)
刊名JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
2014
卷号136期号:10页码:3768-3771
学科分类Chemistry
DOI10.1021/ja5001517
英文摘要Stable porous ionic liquid-water gel induced by inorganic salts was created for the first time. The porous gel was used to develop a one-step method to synthesize supported metal nanocatalysts. Au/SiO2, Ru/SiO2, Pd/Cu(2-pymo)(2) metal-organic framework (Cu-MOF), and Au/polyacrylamide (PAM) were synthesized, in which the supports had hierarchical meso- and macropores, the size of the metal nanocatalysts could be very small (<1 nm), and the size distribution was very narrow even when the metal loading amount was as high as 8 wt %. The catalysts were extremely active, selective, and stable for oxidative esterification of benzyl alcohol to methyl benzoate, benzene hydrogenation to cyclohexane, and oxidation of benzyl alcohol to benzaldehyde because they combined the advantages of the nanocatalysts of small size and hierarchical porosity of the supports. In addition, this method is very simple.
收录类别SCI
WOS记录号WOS:000332922600015
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被引频次:47[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/225172
专题中国科学院高能物理研究所_多学科研究中心_期刊论文
中国科学院高能物理研究所_多学科研究中心
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Kang, XC,Zhang, JL,Shang, WT,et al. One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2014,136(10):3768-3771.
APA Kang, XC.,Zhang, JL.,Shang, WT.,Wu, TB.,Zhang, P.,...&邢雪青.(2014).One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,136(10),3768-3771.
MLA Kang, XC,et al."One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 136.10(2014):3768-3771.
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