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One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel
Kang, XC; Zhang, JL; Shang, WT; Wu, TB; Zhang, P; Han, BX; Wu, ZH; Mo, G; Xing, XQ;吴忠华; Mo G(默广); Xing XQ(邢雪青)
2014
发表期刊JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷号136期号:10页码:3768-3771
摘要Stable porous ionic liquid-water gel induced by inorganic salts was created for the first time. The porous gel was used to develop a one-step method to synthesize supported metal nanocatalysts. Au/SiO2, Ru/SiO2, Pd/Cu(2-pymo)(2) metal-organic framework (Cu-MOF), and Au/polyacrylamide (PAM) were synthesized, in which the supports had hierarchical meso- and macropores, the size of the metal nanocatalysts could be very small (<1 nm), and the size distribution was very narrow even when the metal loading amount was as high as 8 wt %. The catalysts were extremely active, selective, and stable for oxidative esterification of benzyl alcohol to methyl benzoate, benzene hydrogenation to cyclohexane, and oxidation of benzyl alcohol to benzaldehyde because they combined the advantages of the nanocatalysts of small size and hierarchical porosity of the supports. In addition, this method is very simple.
学科领域Chemistry
DOI10.1021/ja5001517
收录类别SCI
WOS记录号WOS:000332922600015
引用统计
被引频次:55[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/225172
专题多学科研究中心
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GB/T 7714
Kang, XC,Zhang, JL,Shang, WT,et al. One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2014,136(10):3768-3771.
APA Kang, XC.,Zhang, JL.,Shang, WT.,Wu, TB.,Zhang, P.,...&邢雪青.(2014).One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,136(10),3768-3771.
MLA Kang, XC,et al."One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 136.10(2014):3768-3771.
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