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High-Pressure-Induced Reversible Phase Transition in Sulfamide
Wang, K; 刘景;Liu, J; Yang, K; Liu, BB; Zou, B
2014
发表期刊JOURNAL OF PHYSICAL CHEMISTRY C
卷号118期号:32页码:18640-18645
摘要Diamond anvil cells combined with Raman spectroscopy and synchrotron X-ray diffraction were used to analyze the compression behavior of sulfamide, a hydrogen-bonded crystal. The marked changes in the Raman spectra at approximately 5 GPa strongly suggest a structural phase transition associated with the rearrangement of hydrogen bonds. Results from angle-dispersive X-ray diffraction confirmed this pressure-induced phase transition, and the high-pressure phase was indexed and refined to a low-symmetry monoclinic structure with space group I2/m. Further phase transitions were not detected up to the maximum pressure of 10 GPa. The observed transition was completely reversible when the pressure was released to ambient conditions. The results from ab initio calculations reveal that the phase transition was mainly caused by changes in the hydrogen-bond networks in sulfamide.
学科领域Chemistry; Science & Technology - Other Topics; Materials Science
DOI10.1021/jp504641z
收录类别SCI
WOS记录号WOS:000340444500043
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被引频次:9[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/225147
专题多学科研究中心
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GB/T 7714
Wang, K,刘景;Liu, J,Yang, K,et al. High-Pressure-Induced Reversible Phase Transition in Sulfamide[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2014,118(32):18640-18645.
APA Wang, K,刘景;Liu, J,Yang, K,Liu, BB,&Zou, B.(2014).High-Pressure-Induced Reversible Phase Transition in Sulfamide.JOURNAL OF PHYSICAL CHEMISTRY C,118(32),18640-18645.
MLA Wang, K,et al."High-Pressure-Induced Reversible Phase Transition in Sulfamide".JOURNAL OF PHYSICAL CHEMISTRY C 118.32(2014):18640-18645.
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