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From antiferromagnetic insulator to correlated metal in pressurized and doped LaMnPO
Simonson, JW; Yin, ZP; Pezzoli, M; Guo, J; Liu, J; Post, K; Efimenko, A; Hollmann, N; Hu, Z; Lin, HJ; Chen, CT; Marques, C; Leyva, V; Smith, G; Lynn, JW; Sun, LL; Kotliar, G; Basov, DN; Tjeng, LH; Aronson, MC;刘景
2012
发表期刊PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA
卷号109期号:27页码:E1815-E1819
摘要Widespread adoption of superconducting technologies awaits the discovery of new materials with enhanced properties, especially higher superconducting transition temperatures T-c. The unexpected discovery of high T-c superconductivity in cuprates suggests that the highest T(c)s occur when pressure or doping transform the localized and moment-bearing electrons in antiferromagnetic insulators into itinerant carriers in a metal, where magnetism is preserved in the form of strong correlations. The absence of this transition in Fe-based superconductors may limit their T(c)s, but even larger T(c)s may be possible in their isostructural Mn analogs, which are antiferromagnetic insulators like the cuprates. It is generally believed that prohibitively large pressures would be required to suppress the effects of the strong Hund's rule coupling in these Mn-based compounds, collapsing the insulating gap and enabling superconductivity. Indeed, no Mn-based compounds are known to be superconductors. The electronic structure calculations and X-ray diffraction measurements presented here challenge these long held beliefs, finding that only modest pressures are required to transform LaMnPO, isostructural to superconducting host LaFeAsO, from an antiferromagnetic insulator to a metallic antiferromagnet, where the Mn moment vanishes in a second pressure-driven transition. Proximity to these charge and moment delocalization transitions in LaMnPO results in a highly correlated metallic state, the familiar breeding ground of superconductivity.
关键词correlated electron systems electronic delocalization transition
学科领域Science & Technology - Other Topics
DOI10.1073/pnas.1117366109
收录类别SCI
WOS记录号WOS:000306641100005
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被引频次:29[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/224368
专题多学科研究中心
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GB/T 7714
Simonson, JW,Yin, ZP,Pezzoli, M,et al. From antiferromagnetic insulator to correlated metal in pressurized and doped LaMnPO[J]. PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,2012,109(27):E1815-E1819.
APA Simonson, JW.,Yin, ZP.,Pezzoli, M.,Guo, J.,Liu, J.,...&Aronson, MC;刘景.(2012).From antiferromagnetic insulator to correlated metal in pressurized and doped LaMnPO.PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA,109(27),E1815-E1819.
MLA Simonson, JW,et al."From antiferromagnetic insulator to correlated metal in pressurized and doped LaMnPO".PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA 109.27(2012):E1815-E1819.
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