Synthesis, structure, photophysics and electrochemiluminescence of Re(I) tricarbonyl complexes with cationic 2,2-bipyridyl ligands
Li, MJ; Liu, X; Shi, YQ; Xie, RJ; Wei, QH; Chen, GN;魏乔华
刊名DALTON TRANSACTIONS
2012
卷号41期号:35页码:10612-10618
学科分类Chemistry
DOI10.1039/c2dt30074e
英文摘要Two water soluble Re(I) tricarbonyl diimine complexes containing cationic 2,2'-bipyridyl ligands [Re(L1)(CO)(3)(AN)](2+) (1) and [Re(L2)(CO)(3)(AN)](3+) (2) (L1 and L2: a cationic 2,2'-bipyridyl ligand, AN: acetonitrile) were synthesized and characterized. Their photophysical, electrochemical and electrochemiluminescent properties were investigated. The crystal structures of the two complexes have also been determined. Electrochemiluminescence (ECL) of the two complexes 1 and 2 have been studied in aqueous buffer solution in the presence of co-reactant tri-n-propylamine (TPrA) or 2-(dibutylamino)-ethanol (DBAE) at a Au working electrode. The ECL behavior of the complexes was also studied in the presence of several surfactants such as Triton X-100 and Zonyl FSN. The ECL signals of the rhenium(I) complex were enhanced about 190-fold and 70-fold at a Au electrode in the presence of Triton X-100 for the [Re(L1)(CO)(3)(AN)](2+)/TPrA and [Re(L1)(CO)(3)(AN)](2+)/DBAE systems, respectively.
收录类别SCI
WOS记录号WOS:000307592600017
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被引频次:9[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/224323
专题中国科学院高能物理研究所_多学科研究中心_期刊论文
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GB/T 7714
Li, MJ,Liu, X,Shi, YQ,et al. Synthesis, structure, photophysics and electrochemiluminescence of Re(I) tricarbonyl complexes with cationic 2,2-bipyridyl ligands[J]. DALTON TRANSACTIONS,2012,41(35):10612-10618.
APA Li, MJ,Liu, X,Shi, YQ,Xie, RJ,Wei, QH,&Chen, GN;魏乔华.(2012).Synthesis, structure, photophysics and electrochemiluminescence of Re(I) tricarbonyl complexes with cationic 2,2-bipyridyl ligands.DALTON TRANSACTIONS,41(35),10612-10618.
MLA Li, MJ,et al."Synthesis, structure, photophysics and electrochemiluminescence of Re(I) tricarbonyl complexes with cationic 2,2-bipyridyl ligands".DALTON TRANSACTIONS 41.35(2012):10612-10618.
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