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Transition-metal distribution in kagome antiferromagnet CoCu3(OH)(6)Cl-2 revealed by resonant X-ray diffraction
Li, YS; 付建龙;吴忠华; Fu, JL; Wu, ZH; Zhang, QM
2013
发表期刊CHEMICAL PHYSICS LETTERS
卷号570页码:37-41
摘要The distribution of chemically similar transition-metal ions is a fundamental issue in the study of herbertsmithite-type kagome antiferromagnets. Using synchrotron radiation, we have performed resonant powder X-ray diffractions on newly synthesized CoCu3(OH)(6)Cl-2, which provide an exact distribution of transition-metal ions in the frustrated antiferromagnet. Both magnetic susceptibility and specific heat measurements are quantitatively consistent with the occupation fractions determined by resonant Xray diffraction. The distribution of transition-metal ions and residual magnetic entropy suggest a novel low temperature (T < 4 K) magnetism, where the interlayer triangular spins undergo a spin-glass freezing while the kagome spins still keep highly frustrated. (c) 2013 Elsevier B.V. All rights reserved.
学科领域Chemistry; Physics
DOI10.1016/j.cplett.2013.03.038
收录类别SCI
WOS记录号WOS:000319102100008
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被引频次:8[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.ihep.ac.cn/handle/311005/223781
专题多学科研究中心
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Li, YS,付建龙;吴忠华,Fu, JL,et al. Transition-metal distribution in kagome antiferromagnet CoCu3(OH)(6)Cl-2 revealed by resonant X-ray diffraction[J]. CHEMICAL PHYSICS LETTERS,2013,570:37-41.
APA Li, YS,付建龙;吴忠华,Fu, JL,Wu, ZH,&Zhang, QM.(2013).Transition-metal distribution in kagome antiferromagnet CoCu3(OH)(6)Cl-2 revealed by resonant X-ray diffraction.CHEMICAL PHYSICS LETTERS,570,37-41.
MLA Li, YS,et al."Transition-metal distribution in kagome antiferromagnet CoCu3(OH)(6)Cl-2 revealed by resonant X-ray diffraction".CHEMICAL PHYSICS LETTERS 570(2013):37-41.
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